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Free clusters and nanoparticles core-level spectroscopy via multi-coincidence electrons and ions detection.

Our aim is to develop new technology to advance beyond the measurement of mass and number concentration of airborne nanoparticles or the determination of their elemental composition and chemical structure, towards real-time access to information on the full-range of  their physical chemistry properties (on the time scale of their agglomerations and transformations).
Advanced light sources in the VUV and XUV are promising facilities to achieve these results owing to the chemical sensitivity and to the local character of the core-level spectroscopy tools to which they provide access. Within the frame of a Long Term proposal accepted by synchrotron radiation facility Elettra, we have developed a UHV apparatus equipped with double-Velocity Map Imaging (VMI) spectrometer for imaging coincidence detection of electrons and ions on a multi-hit detector (MCP with triple- delay-line anode). The apparatus, after being commissioned on November 2017 with XAS and PES measurements on free Ti and V clusters, is fully operational and open to external users proposals.
This Project is pursued in collaboration with the SQS instrument research team at XFEL and with the GasPhase@Elettra and LDM@FERMI joint research group.

Referent: Paolo Piseri

Participants: Paolo Piseri, Claudio Piazzoni